While I opted for replacement of the whole transmission to a '72 C4, the green dot can be modified plenty easily. A later valve body, a better intermediate shift servo, and a higher stall converter are popular upgrades. A set of better clutches and bands will also help quicken shifts over stock, and the originals are likely due for replacement anyways.
Some more advanced mods include drilling the governor weights to raise the full-throttle auto shift points, and adding roller thrust bearings from a (gasp!) TH350 to reduce power loss and fuel consumption, but both of those options require machining. If you don't have a mill or a lathe and some good bits or other tooling, you'll have to farm that work out to a machine shop. Not super expensive, but probably time consuming.
This website has some good material for how to rebuild and do some basic upgrades to the C4.